To clarify, I'm aware that pihole is not intended to run on a client OS, and doesn't monitor at a process level. I'm focused on the intended effect rather than the process itself (blocking malicious/ad servers). And I think I framed my initial question incorrectly as if LS and PiHole as subtitutes. It's perfectly fine and even preferrable to use both as layered protection. I'm just thinking however when it comes for bang-for-buck it seems like PiHole is the better value proposition if you could only set up one.

pi.hole is primarily billed as an ad blocker, but the fundamental way it works is by applying a curated set of DNS lists that are blocked (commonly telemetry and ad servers), and the admin dashboard which is just a web page (therefore works on all platforms, smartphones included) will do the same thing: it tells you every call that every app on every device on your network is making, and you can approve or deny it. You can curate your own list as well and block servers/connections you don't want on the network.

LS afaik operates in the same area where it's intended to be used for privacy. I guess I could see it being useful for people who don't have admin access to their router, but for people who do have such access I would think the benefits of network-wide DNS monitoring/blocking would outweight the costs of having to configure your router settings.

LS seems to not be claiming any security promise on Linux because it can't make any guarantees given eBPF limitations. But the entire purpose is different and there is very little overlap in my view. PiHole is entirely (I think?) just applying the blocklist made easy. LS allows you to build the blocklist in real time.

I would guess that to the extent the blocklists include things that are loaded by applications and not websites, they are almost entirely built by users of something like LittleSnitch or OpenSnitch. This is also entirely doable with wireshark logs, but I think that requires more infrastructure to build into usable lists.

Some telemetry uses hardcoded addresses when DNS doesn't work.

Some telemetry might not be recognized by pi-hole as it is new or has nothing to do with ads.